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Various overoxidized poly(1H-pyrrole) (PPy), poly(N-methylpyrrole) (PMePy) or poly(3,4-ethylenedioxythiophene) (PEDOT) membranes incorporated into an acrylate-based solid polymer electrolyte matrix (SPE) were directly electrosynthesized by a two-step in situ procedure. The aim was to extend and improve fundamental properties of pure SPE materials. The polymer matrix is based on the cross-linking of glycerol propoxylate (1PO/OH) triacrylate (GPTA) with poly(ethylene glycol) diacrylate (PEGDA) and lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) as a conducting salt. A self-standing and flexible polymer electrolyte film is formed during the UV-induced photopolymerization of the acrylate precursors, followed by an electrochemical polymerization of the conducting polymers to form a 3D-IPN. The electrical conductivity of the conducting polymer is destroyed by electrochemical overoxidation in order to convert the conducting polymer into an ion-exchange membrane by introduction of electron-rich groups onto polymer units. The resulting polymer films were characterized by scanning electron microscopy, cyclic voltammetry, electrochemical impedance spectroscopy, differential scanning calorimetry, thermal analysis and infrared spectroscopy. The results of this study show that the combination of a polyacrylate-matrix with ion selective properties of overoxidized CPs leads to new 3D materials with higher ionic conductivity than SPEs and separator or selective ion-exchange membrane properties with good stability by facile fabrication.
The objective of this review is a global assessment of the economics of second‐generation biorefineries, with a focus on the use of food waste and agricultural residues for chemical production by applying biotechnological processes. Analyses are conducted on feedstock and product distribution, applied economic models, and profitability figures for the period 2013–2018. In a study of 163 articles on different biorefinery systems, the production of chemicals is identified as the second major product class, after bioenergy. Bagasse and straw are frequently analyzed second‐generation feedstocks. Based on the evaluation of 22 articles, second‐generation biorefineries producing chemicals by applying biotechnological processes proves to be economically feasible. On average, both the internal rate of return (IRR) and the return on investment (ROI) are 20% and the payback period (PP) is 6 years. The cost share of feedstock in biorefineries is between 0–50%. The price of the end product and the fermentation yields have the most impact on profitability. The processing of food waste that has industrial and municipal origins appears more economical than the processing of agricultural residues. Scientists, policy makers and entrepreneurs with an appropriate risk tolerance are advised to pay particular attention to municipal food waste and the potential economic production of carboxylic acids. For various economic issues related to biorefineries, dynamic‐deterministic models are recommended, which can be extended by a stochastic model. This review provides an initial overview of the economic feasibility of second‐generation biorefineries. Further techno‐economic analyses are required to produce statistically significant statements on key profitability figures. © 2020 The Authors. Biofuels, Bioproducts, and Biorefining published by Society of Chemical Industry and John Wiley & Sons, Ltd.
Hintergrund Die physiotherapeutische Dokumentation spielt im Therapieprozess eine wichtige Rolle, erfolgt jedoch auf unterschiedlichste Weise. Es existieren derzeit eine Vielzahl von Softwarelösungen für die physiotherapeutische Dokumentation, welche sich jedoch in ihren Funktionalitäten stark unterscheiden. Ziel Mithilfe einer Befragung soll ein Konsens von Expertenaus der Physiotherapie im Themengebiet der softwarebasierten Dokumentation ermittelt werden. Anhand der Ergebnisse wird ein Anforderungskatalog für die Entwicklung einer neuartigen und benutzerorientierten Dokumentationssoftware erstellt. Methode Online-Delphi-Befragung mit neun Experten über drei Befragungswellen.
Ergebnisse Hinsichtlich der Anforderungen an die Anamnese konnte ein Konsens erzielt werden. Bei der Gliederung des Befundes kam es zu keiner Übereinstimmung der Experten. Das Ergebnis lässt sich durch unterschiedliche manualtherapeutische Konzepte erklären, die für die Befunderhebung verwendet wurden. Schlussfolgerung Eine softwarebasierte Dokumentation sollte standardisierter als bisher erfolgen, um den ClinicalReasoning-Prozess zu unterstützten. Gleichzeitig ist dabei eine gewisse Flexibilität geboten. Die gesammelten Anforderungen können für die Entwicklung einer neuartigen und benutzerorientierten mobilen Anwendung zur Effizienzsteigerung in der physiotherapeutischen Dokumentation verwendet werden.