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Institute
Stainless steel made to rust: a robust water-splitting catalyst with benchmark characteristics
(2015)
The oxygen evolution reaction (OER) is known as the efficiency-limiting step for the electrochemical cleavage of water mainly due to the large overpotentials commonly used materials on the anode side cause. Since Ni–Fe oxides reduce overpotentials occurring in the OER dramatically they are regarded as anode materials of choice for the electrocatalytically driven water-splitting reaction. We herewith show that a straightforward surface modification carried out with AISI 304, a general purpose austenitic stainless steel, very likely, based upon a dissolution mechanism, to result in the formation of an ultra-thin layer consisting of Ni, Fe oxide with a purity >99%. The Ni enriched thin layer firmly attached to the steel substrate is responsible for the unusual highly efficient anodic conversion of water into oxygen as demonstrated by the low overpotential of 212 mV at 12 mA cm−2 current density in 1 M KOH, 269.2 mV at 10 mA cm−2 current density in 0.1 M KOH respectively. The Ni, Fe-oxide layer formed on the steel creates a stable outer sphere, and the surface oxidized steel samples proved to be inert against longer operating times (>150 ks) in alkaline medium. In addition Faradaic efficiency measurements performed through chronopotentiometry revealed a charge to oxygen conversion close to 100%, thus underpinning the conclusion that no “inner oxidation” based on further oxidation of the metal matrix below the oxide layer occurs. These key figures achieved with an almost unrivalled-inexpensive and unrivalled-accessible material, are among the best ever presented activity characteristics for the anodic water-splitting reaction at pH 13.
Soil versus foliar iodine fertilization as a biofortification strategy for field-grown vegetables
(2015)
Iodine (I) biofortification of vegetables by means of soil and foliar applications was investigated in field experiments on a sandy loam soil. Supply of iodine to the soil in trial plots fertilized with potassium iodide (KI) and potassium iodate directly before planting (0, 1.0, 2.5, 7.5, and 15 kg I ha-1) increased the iodine concentration in the edible plant parts. The highest iodine accumulation levels were observed in the first growing season: In butterhead lettuce and kohlrabi the desired iodine content [50–100 μg I (100 g FM)-1] was obtained or exceeded at a fertilizer rate of 7.5 kg IO3--I ha-1 without a significant yield reduction or impairment of the marketable quality. In contrast, supplying KI at the same rate resulted in a much lower iodine enrichment and clearly visible growth impairment. Soil applied iodine was phytoavailable only for a short period of time as indicated by a rapid decline of CaCl2-extractable iodine in the top soil. Consequently, long-term effects of a one-time iodine soil fertilization could not be observed. A comparison between the soil and the foliar fertilization revealed a better performance of iodine applied aerially to butterhead lettuce, which reached the desired iodine accumulation in edible plant parts at a fertilizer rate of 0.5 kg I--I ha-1. In contrast, the iodine content in the tuber of sprayed kohlrabi remained far below the targeted range. The results indicate that a sufficient spreading of iodine applied on the edible plant parts is crucial for the efficiency of the foliar approach and leafy vegetables are the more suitable target crops. The low iodine doses needed as well as the easy and inexpensive application may favor the implementation of foliar sprays as the preferred iodine biofortification strategy in practice.
Mit einem systematischen Ansatz konnte basierend auf gering aufgelösten Daten (Bodenkarte, Höhenmodell, Landnutzungsklassifikation) das theoretische Expansionspotential für Ackerflächen in der Provinz Tjumen (Westsibirien, Russische Föderation) abgeschätzt werden. Die theoretisch mögliche Ausdehnung der Ackernutzung um 57% in den landwirtschaftlich relevanten Gebieten konnte allerdings nur zur Hälfte mit Groundtruthdaten in 3 Testareas (je 400 km²) validiert werden. Darüber hinaus waren 52% dieser positiven Validierungspunkte auf Ackerbrachen verortet, die derzeit nicht ökonomisch rentabel zu bewirtschaften sind. Insgesamt kann daher nur eine Expansion der Ackerflächen um 14,5% (? 1900 km² bzw. 1,1% der Gesamtfläche) als potentiell möglich angesehen werden.
Dieses Buch gibt einen Überblick über das Controlling als wichtiges System innerhalb des Krankenhaus-Managements. Controlling wird als eine betriebswirtschaftliche Teildisziplin dargestellt, die vor allem im Gesundheitsbereich Daten, Analysen und Auswertungen für Nicht-Ökonomen bereitstellt. Das Werk bereitet aktuelle Forschungsansätze für die Praxis auf, um darauf aufbauend anwendungsorientierte Controllinginstrumente vorzustellen, die mit Daten und Zahlen aus der Praxis hinterlegt sowie beispielhaft erläutert sind.
Vergleich der Effekte eines funktionellen Stabilisations- mit einem Standardtraining auf Schmerz, Funktion, Kinematik der unteren Extremität und des Rumpfes, Ausdauerfähigkeit der Rumpfmuskulatur und der Kraft der exzentrischen Kniegelenks- und Hüftmuskultur bei Frauen mit patellofemoralen Schmerzen.